Description processes of the interaction of water and aqueous solutions with fuel-containing materials in the New Safe Confinement of the “Shelter” object

M. Tokarchuk; B. Markovych; O. Zakharyash; O. Ivankiv; S. Mokhniak

doi:10.5488/cmp.28.11601

Authors

M. Tokarchuk Institute for Condensed Matter Physics of the National Academy of Sciences of Ukraine, 1 Svientsitskii Str., 79011 Lviv, Ukraine; Lviv Polytechnic National University, 12 S. Bandera Str., 79013 Lviv, Ukraine https://orcid.org/0000-0002-9205-1790
B. Markovych Lviv Polytechnic National University, 12 S. Bandera Str., 79013 Lviv, Ukraine https://orcid.org/0000-0002-8813-9108
O. Zakharyash Lviv Polytechnic National University, 12 S. Bandera Str., 79013 Lviv, Ukraine https://orcid.org/0000-0002-3083-9478
O. Ivankiv Institute for Condensed Matter Physics of the National Academy of Sciences of Ukraine, 1 Svientsitskii Str., 79011 Lviv, Ukraine
S. Mokhniak Lviv Polytechnic National University, 12 S. Bandera Str., 79013 Lviv, Ukraine https://orcid.org/0009-0008-3246-2070

DOI:

https://doi.org/10.5488/cmp.28.11601

Keywords:

diffusion, porous medium, hydrolysis, reactions, adsorption

Abstract

The main mechanisms and conditions of interaction of lava-like fuel-containing materials (LFCM) with the atmosphere, water and aqueous solutions are presented. The mechanisms of destruction of the LFCM surface, including ion-exchange processes, hydrolysis, dissolution, oxidation, etc., were analyzed. Inhomogeneous diffusion coefficients for UO₂²⁺, Cs⁺ ions at the interface “aqueous solution of radioactive elements – LFCM” were calculated. The interdiffusion processes and the rate of penetration into the porous medium of the reaction front of the internal hydrolysis of the silicon-oxygen network during interaction with an aqueous solution were analyzed, where the reaction and adsorption processes are hidden in the rate of internal hydrolysis.

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